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Free, publicly-accessible full text available June 9, 2026
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Tyson, Trevor A; Amarasinghe, Sandun; Abeykoon, A_M Milinda; Lalancette, Roger; Du, Kai; Fang, Xiaochen; Cheong, Sang-W; Al-Mahboob, Abdullah; Sadowski, Jerzy T (, 2D Materials)Abstract The surface magnetization of Fe3GeTe2was examined by low-energy electron microscopy (LEEM) using an off-normal incidence electron beam. We found that the 180° domain walls are of Bloch type. Temperature-dependent LEEM measurements yield a surface magnetization with a surface critical exponentβ1 = 0.79 ± 0.02. This result is consistent with surface magnetism in the 3D semi-infinite Heisenberg (β1 = 0.84 ± 0.01) or Ising (β1 = 0.78 ± 0.02) models, which is distinctly different from the bulk exponent (β= 0.34 ± 0.07). The measurements reveal the power of LEEM with a tilted beam to determine magnetic domain structure in quantum materials without the need for the use of spin-polarized electrons. Single crystal diffraction measurements reveal inversion symmetry-breaking weak peaks and yield space group P-6m2. This Fe site defect-derived loss of inversion symmetry enables the formation of skyrmions in this Fe3GeTe2crystal.more » « lessFree, publicly-accessible full text available February 24, 2026
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